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Radionuclide Migration

The unexpected behavior of radionuclides in the subsurface near the ChNPP has challenged common wisdom to search for the mechanisms responsible for rapid migration of the pollutants into the groundwater system. Field observations and results of preliminary modeling show the important role played by surface depression zones as areas of anomalously rapid vertical radionuclide migration to the shallow water table. Depression zones have hydrogeological, geophysical, and geochemical properties that apparently provide preferential vertical conduits for water and dissolved contaminants to migrate into the subsurface.

The depression zones are "collectors" of radionuclides as overland flow to these zones mobilizes surface sediments and associated radionuclides that are then redeposited in the depressions. Consequently, the surface depressions, while inducing shallow groundwater contamination, may be beneficial in removing, or scavenging, radionuclides from the landscape. Over time a non-point source pollution problem is being naturally converted into a finite number of point sources of contamination. Figure 1 shows a schematic representation of a typical depression zone and the associated surface catchment area.

Many depression zones occur within the Chernobyl Exclusion Zone. They are typically round, elliptical, or irregular in shape with dimensions ranging from several tens of meters to several hundred meters in diameter and 3 m to 10 m in depth. They cover about 10% of the CEZ area, though they influence the distribution of over 60% of surface runoff. Several of the depression zones have been instrumented, sampled, and geophysically surveyed by Radioecology Center scientists to better document their behavior. Radionuclide assessments within these vertical pathways suggest that the surface depression zones may be responsible for penetration of a significant portion of initial and subsequent surface radioactive contamination into shallow aquifers. In order to understand this hydraulic and geochemical phenomenon, the vertical mass flux (water and radionuclides) must be documented as to chromatographic effects, speed of the migration, effects of organic adsorption, and changes controlled by rock characteristics and clay mineralogy along with other specific information. The depression zones are sources of contamination for aquifers from which water has been extracted for use in and around the Chernobyl area.

Rock properties are anomalous in these rapid migration zones because of possible tectonic dislocations, fracturing, or disintegration of rock materials that appear often as complex and dense networks. Originally the depression zones may have been formed as kettles that are characteristic of glaciated terrain but possibly were complicated by zones of weakness that have become faults. They could be activated under influence of suffosion, or other processes. In karst areas in other parts of the world, such zones are easily recognized and have been extensively studied. Much less documented are zones within unconsolidated or highly plastic terrigenous (sandy or clay) rocks, such as those prevalent in the Chernobyl area. The depression zones are easily identified by geophysical data (Figure 2).

A more thorough understanding of the physical and chemical behavior of surface depression zones in the Chernobyl area is critically important for several reasons. First, there are significant geotechnical implications for depression zones related to radioactive waste storage and burial associated with the continuing aftermath of the Chernobyl accident. Second, the migration of Cs and 137 Sr to shallow groundwater within the Chernobyl Exclusion Zone poses an immediate threat to local, 90 rural water supplies. Third, there is a long-term health risk posed to a large population (i.e., +2 million)

Figure 1. Schematic representation of a typical depression zone near the Chernobyl NPP. 
(Source: Shestapalov, V.M., and A.S. Bohuslavsky. 2002. "Chernobyl Disaster and Groundwater." A.A. Balkema, Tokyo,  pp.2001-253;
Shestapalov, V.M.,(ed). 2001. "Water Cycle in Hydrogeological Structures and Chernobyl Disaster."  Vol. 1, Kiev, p.242 )

 

Figure 2. A section of the shallow deposits of a depression within the Chernobyl Exclusion Zone imaged by high-frequency (300 MHz) electromagnetic sensing equipment (SIR-2): Depth = surface to 4 m. Width = 60 m. The depression zone is evident in the center. persons) via the Kiev water supply from migration of radionuclides of Chernobyl origin to regional groundwater resources through depression zones.
(Source: Shestapalov, V.M., and A.S. Bohuslavsky. 2002. "Chernobyl Disaster and Groundwater." A.A. Balkema, Tokyo,  pp.2001-253;
Shestapalov, V.M.,(ed). 2001. "Water Cycle in Hydrogeological Structures and Chernobyl Disaster."  Vol. 1, Kiev, p.242 )


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